This program focused on fundamental investigations of mixing, chemical-reaction, and combustion processes, in turbulent, subsonic, and supersonic free-shear flows. The program was comprised of an experimental effort; an analytical, modeling, and computational effort; and a diagnostics, instrumentation, and data-acquisition-development effort, with significant progress in each. With regard to gas-phase shear-layer mixing and combustion, effects of inflow/initial conditions, compressibility, and Reynolds number were experimentally investigated and, to a large extent, clarified. New measures to characterize level sets in turbulence were developed and successfully employed to characterize experimental data of liquid-phase turbulent-jet flows as well as three-dimensional direct-numerical-simulation data of Rayleigh-Taylor-instability flows. The computational effort has added to our understanding of the (H2+NO)/F2 chemical system employed in the shear-layer-mixing investigations as well as mixing in high-speed flows, along with further developments in Riemann-Invariant-Manifold gasdynamic simulation techniques and their application to unsteady detonation phenomena. On the diagnostic front, developments in digital imaging and Image Correlation Velocimetry have continued, and been used to investigate turbulent-jet mixing, the unsteady flow over an accelerating airfoil, to mitigate aliasing problems in the computer reconstruction of (2+1)-dimensional isosurface data, and in other applications.