Attosecond Experiments on Plasmonic Nanostructures

Attosecond Experiments on Plasmonic Nanostructures
Author: Johannes Schötz
Publisher: Springer
Total Pages: 115
Release: 2016-04-13
Genre: Science
ISBN: 3658137134

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Johannes Schötz presents the first measurements of optical electro-magnetic near-fields around nanostructures with subcycle-resolution. The ability to measure and understand light-matter interactions on the nanoscale is an important component for the development of light-wave-electronics, the control and steering of electron dynamics with the frequency of light, which promises a speed-up by several orders of magnitude compared to conventional electronics. The experiments presented here on metallic nanotips, widely used in experiments and applications, do not only demonstrate the feasibility of attosecond streaking as a unique tool for fundamental studies of ultrafast nanophotonics but also represent a first important step towards this goal.

Attosecond Nanophysics

Attosecond Nanophysics
Author: Peter Hommelhoff
Publisher: John Wiley & Sons
Total Pages: 392
Release: 2015-03-09
Genre: Science
ISBN: 3527411712

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Die Autoren geben einen tiefen wie auch umfassenden Überblick über die aktuelle Forschung im Bereich der Attosekunden-Nanophysik, d.h. einem Gebiet der nanoskaligen Festkörpersysteme und der natürlichen Zeitskala von Elektronenbewegungen.

Dissipative Quantum Mechanics of Nanostructures

Dissipative Quantum Mechanics of Nanostructures
Author: Andrei D. Zaikin
Publisher: CRC Press
Total Pages: 957
Release: 2019-05-24
Genre: Science
ISBN: 1000023664

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Continuing miniaturization of electronic devices, together with the quickly growing number of nanotechnological applications, demands a profound understanding of the underlying physics. Most of the fundamental problems of modern condensed matter physics involve various aspects of quantum transport and fluctuation phenomena at the nanoscale. In nanostructures, electrons are usually confined to a limited volume and interact with each other and lattice ions, simultaneously suffering multiple scattering events on impurities, barriers, surface imperfections, and other defects. Electron interaction with other degrees of freedom generally yields two major consequences, quantum dissipation and quantum decoherence. In other words, electrons can lose their energy and ability for quantum interference even at very low temperatures. These two different, but related, processes are at the heart of all quantum phenomena discussed in this book. This book presents copious details to facilitate the understanding of the basic physics behind a result and the learning to technically reproduce the result without delving into extra literature. The book subtly balances the description of theoretical methods and techniques and the display of the rich landscape of the physical phenomena that can be accessed by these methods. It is useful for a broad readership ranging from master’s and PhD students to postdocs and senior researchers.

Electron Transport in Nanostructures and Mesoscopic Devices

Electron Transport in Nanostructures and Mesoscopic Devices
Author: Thierry Ouisse
Publisher: John Wiley & Sons
Total Pages: 282
Release: 2013-03-01
Genre: Technology & Engineering
ISBN: 111862338X

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This book introduces researchers and students to the physical principles which govern the operation of solid-state devices whose overall length is smaller than the electron mean free path. In quantum systems such as these, electron wave behavior prevails, and transport properties must be assessed by calculating transmission amplitudes rather than microscopic conductivity. Emphasis is placed on detailing the physical laws that apply under these circumstances, and on giving a clear account of the most important phenomena. The coverage is comprehensive, with mathematics and theoretical material systematically kept at the most accessible level. The various physical effects are clearly differentiated, ranging from transmission formalism to the Coulomb blockade effect and current noise fluctuations. Practical exercises and solutions have also been included to facilitate the reader's understanding.

Strong-field and Time-resolved Photoemission from Plasmonic Nanoparticles

Strong-field and Time-resolved Photoemission from Plasmonic Nanoparticles
Author: Erfan Saydanzad
Publisher:
Total Pages: 0
Release: 2022
Genre:
ISBN:

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In this dissertation, numerical models have been developed to investigate strong-field photoemission and attosecond streaking spectroscopy from plasmonic nanoparticles. Attosecond streaking spectroscopy and strong-field photoemission are powerful methods for investigating the electronic dynamics in gaseous atoms, that are currently being transferred to the investigation of collective electronic (plasmonic) effects in solids and nanostructures. First, a classical model is proposed to study plasmon excitations in metal nanoparticles using attosecond streaking spectroscopy. In this model, by sampling over classical photoelectron trajectories, we simulated streaked photoelectron energy spectra as a function of the time delay between ionizing isolated attosecond extreme ultraviolet pulses and assisting infrared or visible streaking laser pulses. Our theoretical model comprises a sequence of four steps: XUV excitation, electron transport in the nanoparticles, escape from the surface of the nanoparticles, and propagation to the photoelectron detector. Based on numerical applications to gold nanospheres, we investigated streaked photoemission spectra with regard to (i) the nanoparticle's dielectric response to the electric field of the streaking laser pulse, (ii) relative contributions of photoelectron release from different locations on and in the nanoparticle, (iii) contributions of photoemission from the Fermi level only versus emission from the entire occupied conduction band, and (iv) their fidelity in imaging the spatiotemporal distribution of the induced plasmonic field near the particle's surface. Second, based on this model, we suggest a method for reconstructing induced plasmonic fields with nm spatial and sub-fs temporal resolution from streaked photoemission spectra. Applying this imaging scheme to gold nanospheres, we demonstrated the accurate spatiotemporal reconstruction of the plasmonic near-field distribution in comparison with the directly calculated plasmonic field. Finally, strong-field photoemission from metal nanoparticles was modeled. The numerical model includes: (i) photoelectron emission on the nanoparticle surface by an intense infrared laser pulse, (ii) photoelectron propagation outside the nanosphere in the presence of the incident laser and induced plasmonic fields, and (iii) photoelectron rescattering and recombination to the nanoparticle. Based on simulated photoelectron-momentum distributions from gold nanospheres for two different intensities, and in comparison with velocity-map-image photoelectron spectra measured at the James R. Macdonald Laboratory, we scrutinize the effects of induced plasmonic fields, photoelectron correlations and electron-residual charge interactions, and photoelectron rescattering and recombination at the nanoparticle surface.

Electrical Transport in Nanoscale Systems

Electrical Transport in Nanoscale Systems
Author: Massimiliano Di Ventra
Publisher: Cambridge University Press
Total Pages: 477
Release: 2008-08-07
Genre: Science
ISBN: 1139475029

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In recent years there has been a huge increase in the research and development of nanoscale science and technology. Central to the understanding of the properties of nanoscale structures is the modeling of electronic conduction through these systems. This graduate textbook provides an in-depth description of the transport phenomena relevant to systems of nanoscale dimensions. In this textbook the different theoretical approaches are critically discussed, with emphasis on their basic assumptions and approximations. The book also covers information content in the measurement of currents, the role of initial conditions in establishing a steady state, and the modern use of density-functional theory. Topics are introduced by simple physical arguments, with particular attention to the non-equilibrium statistical nature of electrical conduction, and followed by a detailed formal derivation. This textbook is ideal for graduate students in physics, chemistry, and electrical engineering.

Collective Plasmon-Modes in Gain Media

Collective Plasmon-Modes in Gain Media
Author: V.A.G. Rivera
Publisher: Springer
Total Pages: 147
Release: 2014-09-03
Genre: Science
ISBN: 3319095250

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This book represents the first detailed description, including both theoretical aspects and experimental methods, of the interaction of rare-earth ions with surface plasmon polariton from the point of view of collective plasmon-photon interactions via resonance modes (metal nanoparticles or nanostructure arrays) with quantum emitters (rare-earth ions). These interactions are of particular interest for applications to optical telecommunications, optical displays, and laser solid state technologies. Thus, our main goal is to give a more precise overview of the rapidly emerging field of nanophotonics by means of the study of the quantum properties of light interaction with matter at the nanoscale. In this way, collective plasmon-modes in a gain medium result from the interaction/coupling between a quantum emitter (created by rare-earth ions) with a metallic surface, inducing different effects such as the polarization of the metal electrons (so-called surface plasmon polariton - SPP), a field enhancement sustained by resonance coupling, or transfer of energy due to non-resonant coupling between the metallic nanostructure and the optically active surrounding medium. These effects counteract the absorption losses in the metal to enhance luminescence properties or even to control the polarization and phase of quantum emitters. The engineering of plasmons/SPP in gain media constitutes a new field in nanophotonics science with a tremendous technological potential in integrated optics/photonics at the nanoscale based on the control of quantum effects. This book will be an essential tool for scientists, engineers, and graduate and undergraduate students interested not only in a new frontier of fundamental physics, but also in the realization of nanophotonic devices for optical telecommunication.